Acousto-optical Research Articles

Acoustic and acousto-optic properties of Ga10Ge15Te75 glass

The acoustic and acousto-optic (AO) properties of the Ga10Ge15Te75 glass, which is promising for creation of AO devices operating with the near and middle infrared optical radiation, are studied. In this paper, the experimental results for the longitudinal and shear acoustic waves phase velocities and the AO figure of merit (M2) in case of isotropic diffraction by these waves are presented. All measurements are carried out for the 3.39 µm optical wavelength. The obtained M2 magnitudes turned out to be close to 1000·10–15s3/kg that significantly exceeds the typical values observed in germanium (Ge) crystal – the basic material for middle infrared AO devices fabrication. The experimentally determined longitudinal acoustic wave attenuation coefficient for 100 MHz ultrasound frequency turns out to be 1.32 ± 0.05 cm-1. Finally, the acoustic and AO properties of telluride based glasses with the close chemical composition, namely Ga10Ge15Te75, Si25Te75 and Ge25Se15Te60 glasses, are compared.

Temperature effect on acoustic waves reflection condition in anisotropic crystals

The reflection of acoustic waves in anisotropic media has found important applications in acousto-optics (AO). It may be realized both with changing the type of acoustic mode and without it. The latter case is applied for the realization of the quasi-collinear AO diffraction geometry for which the incident light and ultrasound wave group velocity vectors are collinear. The acoustic wave involved into the AO interaction exists due to the reflection from the AO cell input optical face. Quasi-collinear configuration of AO interaction enables achieving exceptionally high spectral resolution and diffraction efficiency, therefore, it is applied for the laser pulse shaping. However, the application of AO tunable filters for such purposes requires high acoustic power values, which induce the temperature gradients in the AO crystal. Temperature variations influence the stiffness constants of the AO crystal, impacting the characteristics of incident and reflected acoustic waves, affecting the acoustic wave reflection condition and consequently, the AO diffraction characteristics. This study presents the theoretical and experimental examination of the temperature influence on the acoustic beam reflection in anisotropic crystals on the example of tellurium dioxide crystal. This paper is supported by the Russian Science Foundation, grant 23-12-00057.

1 kHz, 5.3 kW peak power pulse generation from a LiNbO3 acousto-optically Q-switched Er:YAP laser

In this paper, we present, for the first time, a bulk LiNbO3 (LN) acousto-optic (AO) Q-switched Er:YAP laser operating at a pulse repetition frequency (PRF) of 1 kHz. At this frequency, the laser achieves a maximum single pulse energy of 0.34 mJ, with a corresponding pulse duration of 64.5 ns and a peak power of 5.3 kW. Additionally, we characterize the laser beam quality factors, Mx2 = 2.7 and My2 = 2.5, and its central wavelength at 2730.7 nm, all at 1 kHz. These results highlight the significant potential of LN AO Q-switched Er:YAP lasers for enhancing mid-infrared laser applications.

Spatial-Dependent Spectral Response of Acousto-Optic Tunable Filters with Inhomogeneous Acoustic Distribution.

The spectral response of an acousto-optic tunable filter (AOTF) is crucial for an AOTF based spectral imaging system. The acousto-optic (AO) interaction within the spatial-distributed area of the acoustic field determines the spectral response of the light incidence. Assuming an ideally uniform acoustic field distribution, phase-matching geometries can be applied to calculate the anisotropic Bragg diffraction in AO interactions, determining the wavelength and direction of the diffracted light. In this ideal scenario, the wavelength of the diffracted light depends solely on the direction of the incident light. However, due to the non-ideal nature of the acoustic field, the wavelength of the diffracted light exhibits slight variations with incident position. In this paper, an analytical model is proposed to calculate the spatial-dependent spectral response of the diffracted light under non-uniform acoustic field distribution. The study computes the variation pattern of the diffracted light amplitude caused by the inhomogeneous acoustic distribution. The theoretical considerations and computational model are confirmed by AOTF frequency scanning experiments. The study demonstrates that the distribution of the acoustic field leads to non-uniform spatial-spectral response in the AOTF, and the spatial AO interaction computational model can provide data support for calibrating AOTF systems in imaging applications.

Temperature impact on acoustic wave reflection in quasi-collinear acousto-optic devices.

Quasi-collinear geometry is a special configuration of acousto-optic (AO) diffraction that applies the acoustic wave reflection from the AO cell input optical face and provides an extremely large interaction length for achieving abnormally high spectral resolution of AO tunable filters. As a result, it becomes possible to implement the multifrequency diffraction which has found important applications for laser pulse shaping. The operation of quasi-collinear AO devices in the multifrequency diffraction regimen is accompanied by the appearance of the longitudinal and transverse temperature gradients in the crystal, mainly due to the acoustic power absorption. Temperature changes the AO cell material stiffness moduli, affecting the characteristics of the incident and reflected acoustic waves (propagation velocities and walk-off angles), and the reflection condition in general. On the example of paratellurite crystal is shown that the AO cell heating near the reflecting facet leads to a deviation of the reflected acoustic beam propagation direction from that specified during the AO cell manufacturing. The deviation magnitude depends on the reflection geometry choice and, in the paratellurite, may exceed several degrees, which adversely affects the AO diffraction characteristics, reducing the AO interaction efficiency and distorting the transmission function shape. The reflected beam deviation may be compensated by means of choosing the angle between the AO cell reflecting face and the piezoelectric transducer face, taking into account the operating AO device thermal regimen.

Achieving high acousto-optic properties and low thermal expansion anisotropy in TeO2 single crystals via Mn-doping

TeO2 single crystals have been widely used in military and civilian fields as an excellent acousto-optic (AO) material. However, due to its significant thermal expansion anisotropy and poor mechanical properties, there is a considerable risk of cracking, which hinders further applications in the AO field. Here we successfully grew a TeO2 single crystal doped with 2 % Mn4+ ions (TeO2:0.02Mn4+). This single crystal demonstrates excellent characteristics, including lower acoustic attenuation (α) and larger refractive index values. In addition, it also possesses a higher AO figure of merit (M2) of 832 × 10−15 s3/kg than TeO2 single crystal (∼793 × 10−15 s3/kg). More importantly, the TeO2:0.02Mn4+ single crystal demonstrates low thermal expansion anisotropy within a temperature range of up to 450 °C, indicating a greater practical value. The high AO performance may be attributed to manganese ion doping. The doping of Mn increased the refractive indices by enhancing the electronic polarizability and achieved lower acoustic attenuation by improving mechanical properties. Combining the results of elastic modulus and Raman spectroscopy analysis, it is observed that manganese doping optimizes crystal structure disorder, thus improving the issue of thermal expansion anisotropy. These results indicate that this TeO2:0.02Mn4+ single crystal has significant potential in designing and manufacturing AO devices.

Concept for power scaling by harmonic beam coaxial combination in an intra-cavity frequency doubling laser.

A new method of harmonic beam coaxial combination (HBCC) from two intra-cavity frequency doubling branches was demonstrated. Firstly, two identical nanosecond (ns) 532 nm green lasers with high power and good beam quality were created. Each green laser was constructed of an intra-cavity frequency doubling branch based on a laser diode (LD) end-pumped acousto-optical (AO) Q-switched 1064 nm Nd:YVO4 laser in a LiB3O5 (LBO) nonlinear crystal. Each branch generated about 45 W green output at a 50 kHz pulse repetition rate (PRR) with diffraction limited beam quality. The first green beam was injected into the LBO crystal in the second branch, and the pulses from the two branches did not exist simultaneously. Then, the HBCC was performed. Consequently, an 83 W combined green output power at 532 nm was obtained with a combination efficiency of 92.2%. The PRR of the HBCC pulse was doubled to be 100 kHz, with a pulse width of about 22 ns, corresponding to a single pulse energy of 0.83 mJ and a peak power of 37.73 kW. The combined beam quality factor was measured to be M x2 = 1.80 in the x direction and M y2 = 1.71 in the y direction, respectively. Moreover, many more beams could also be combined with this method for further scaling the green power.

Phase-tuned acousto-optic spatial filter.

An acousto-optic (AO) tunable filter with a phase-controlled dual-section piezoelectric transducer is designed and created for laser beam shaping (LBS). Owing to the acoustic beam steering effect, we experimentally observe splitting of the two-dimensional transfer function. As a result, we demonstrate generation of tunable bottle laser beams and dual-ring intensity distributions for the diffracted beam.

Polymer-dispersed liquid-crystal coatings for ultrasound visualization: Experiment and theory.

Polymer dispersed liquid crystal (PDLC) films are formed of droplets of liquid crystal (LC) held in a polymer matrix. Similar to aligned LC films, PDLCs exhibit the acousto-optic (AO) effect when excited by acoustic waves of sufficient amplitude, whereby the PDLC film becomes transparent in the excited regions (acoustic clearing). Despite decades of research there is still debate over the mechanisms of the AO effect for the case of LC films, with several competing theories, and AO effects in PDLC have not been studied theoretically. This paper explores the AO effect in PDLC both experimentally and theoretically, and attempts a theoretical description of the observed phenomena based on the theoretical approach by Selinger etal. for aligned LC films. The acousto-optic effect in PDLC is shown to be due to direct interaction of acoustic waves with LC droplets, rather than due to compression of the droplet itself. Polarizing microscopy revealed changes in droplet shape at excited points. This is consistent with reorientation as a contributing factor, possibly coexisting with flows at higher excitation powers. In previous experimental studies PDLC films were prepared with cover slides, in the same way as LC AO cells, significantly limiting applications by adding complexity to the design. Also, to exhibit AO clearing it was considered that the PDLC needed to be prepared with high LC concentrations (over 75% by weight). We demonstrate that no cover slide is necessary, and that PDLC coatings without a cover have improved sensitivity to acoustic waves. We demonstrate the AO effect for LC concentrations as low as 40% by weight. The ability to use standard composition PDLC, with no top cover, is paving the way to paint-on visual ultrasound sensors.

Lithium niobate on insulator – fundamental opto-electronic properties and photonic device prospects

Abstract Lithium niobate on insulator (LNOI) combines a variety of optoelectronic properties and can meet practical performance requirements that are uncommon in optoelectronic materials. This review introduces the fundamentals and the photonic device concepts that arise from the LNOI materials platform. Firstly, the nonlinear optical response of LNOI is presented, including birefringent phase matching (BPM), modal phase matching (MPM), and quasi-phase matching (QPM). The tunable properties are also introduced, including electro-optical (EO), thermo-optical (TO), and acousto-optical (AO) effects. The structures of nonlinear optical devices, such as ridge waveguides (including periodically polarized inversion waveguides), Mach–Zehnder interferometer (MZI) modulators and micro-resonators (such as disks and rings) are demonstrated. Finally, the future of LNOI devices is discussed. In the already mature and developed optoelectronic material systems, it is rare to find one particular material system supporting so many basic optical components, photonic devices and optoelectronic devices as LNOI does in the field of integrated photonic chips.

Correlation between composition, structure, and acousto-optic properties of As100-xSx chalcogenide glasses

Acousto-optic (AO) devices have great application potential in laser technology and network communication. Chalcogenide (ChG) glass is promising for AO devices because of its excellent infrared transparency and high AO figure of merit. Among them, As–S glasses represent the most typical and extensively studied ChG system. However, the correlation between the network structure of As–S glasses in the As-rich and S-rich regions and their AO properties remains to be investigated. In this work, the effect of glass composition and glass structure on the AO properties of As–S glasses was investigated. The gradual formation of homopolar As–As and S–S bonds leads to the weakening of the network crosslinking degree of the glass structure in the vicinity of As-rich and S-rich regions, which results in a reduction in the AO properties. In particular, the presence of long-chain As–S–As bonds in the As40S60 glass primarily causes its superior AO properties. The above results provide an important reference for the further investigation on the correlation between glass composition, structure, and AO properties and the development of As–S based AO media and devices.

Interstitial doping of Mn4+ ions: An effective method to optimize the optical properties of TeO2 single crystal

AbstractTeO2 single crystal has drawn much attention in recent years due to its excellent acousto‐optic (AO) performance in the field of spectral imaging and optical processing. The optical properties of TeO2 single crystal are critical for the fabrication of AO devices. To improve the optical properties of the TeO2 single crystal, Mn4+ ions were doped into the TeO2 lattice. Herein, bulk TeO2 single crystal and TeO2:0.02Mn4+ single crystal have been successfully grown by a Bridgman method. Compared with the TeO2 single crystal, a 30% transmittance increase was observed in the TeO2:0.02Mn4+ single crystal. Furthermore, the TeO2:0.02Mn4+ single crystal shows a smaller extinction coefficient (≤0.01) in the Vis–NIR region, indicating less optical loss. The bandgap energy of TeO2:0.02Mn4+ was broadened from 3.360 to 3.635 eV. In addition, TeO2:0.02Mn4+ single crystal exhibits a higher refractive index (about 2.244), which indicates that TeO2:0.02Mn4+ single crystal is a potential medium for high‐efficiency AO devices.

Continuous wave and active Q-switched operation of Watt-level LED-pumped two-rod Nd,Ce:YAG laser

Abstract In this paper, we demonstrated a high-performance LED-side-pumped two-rod Nd,Ce:YAG laser with continuous-wave (CW) and acousto-optical (A-O) Q-switched operation. A symmetrical shaped flat-flat cavity with two identical LED-side-pumped laser modules was employed for power scalability. In the CW regime, the maximum output average power of laser at 1064 nm was 4.41 W, corresponding to the highest optical conversion efficiency of 5.3% and a slope efficiency of 12.4%. In the active Q-switched regime, the pulse energy of laser was as high as 0.89 mJ at a repetition rate of 800 Hz with a pulse width of 457.2 ns, corresponding to the highest peak output power was 1.94 kW and the M2 factor was measured to be about 8.8. To the best of our knowledge, this is the first demonstration and the highest performance of an CW LED-side-pumped two-rod laser Nd,Ce:YAG with watt-level output reported so far.

An LED-Side-Pumped Intracavity Frequency-Doubled Nd,Ce:YAG Laser Producing a 2W Q-Switched Red Beam

We report a high-average-power acousto-optic (AO) Q-switched intracavity frequency-doubled red laser based on a high-efficiency light-emitting-diode (LED) pumped two-rod Nd,Ce:YAG laser module. Under quasi-continuous wave operation conditions, a maximum output power of 1319.08 nm wavelength was achieved at 11.26 W at a repetition rate of 100 Hz, corresponding to a maximum optical efficiency of 13.9% and a slope efficiency of 17.9%. In the active Q-switched regime, the pulse energy of the laser was as high as 800 μJ at a repetition rate of 10 kHz with a pulse width of 1.5 μs. Under non-critical phase-matched KTP crystal conditions, an average power of 2.03 W of 658.66 nm through intracavity frequency-doubling was obtained at a repetition frequency of 10 kHz with a duration of 1.3 μs, and the M 2 factor was measured to be about 5.8. To the best of our knowledge, this is the highest average power of an LED-pumped AO Q-switched 1319 nm laser and intracavity frequency-doubled red laser reported to date.

Characterization of flexural acoustic waves in optical fibers using a fiber-tip interferometer

An experimental study using a fiber-tip interferometer (FTI) to characterize traveling flexural acoustic waves (TFAWs) along an optical fiber is reported. The measurements carried out with the FTI are performed following two different procedures: one of them relies on adjusting the interferometer at the quadrature condition and the other extracts the information from the amplitudes of the fundamental and second harmonic of the interference signal. From our measurements, the detection limit of the FTI is 0.5 nm and the upper limit of the linear regime is 30 nm. These results validate the use of the FTI to detect nanometric displacements associated to the amplitude of acoustic waves along an optical fiber. Parameters such as the acoustic wavelength, attenuation coefficient, and phase velocity are measured for a range of acoustic frequencies around the 2 MHz region. Furthermore, and supported by the in-fiber acousto-optic (AO) effect produced by TFAWs, parameters associated to an acoustic wave packet such as the group velocity and the group attenuation coefficient are also determined. This set of experimental results provide useful information of the mechanisms underlying the propagation of TFAWs along an optical fiber and its corresponding AO effect.

Angular-Spectral Characteristics of Acousto-Optic Tunable Filters Based on Mercurous Halide Crystals.

The angular and spectral properties crucial for the functionality of acousto-optic (AO) devices are determined by phase-matching geometries in AO interactions. In applications such as spectral imagers based on acousto-optic tunable filters (AOTFs), systematic throughput is constrained by the angle separating diffracted and transmitted light. This research introduces an analytical model that elucidates the angular-spectral properties of diffracted beams in mercurous halide crystals. These crystals possess a wide transmissive spectral range, from visible light to long-wave infrared light. The study computes and confirms correlations between the separation angle and parameters including incident angle, polarization, acoustic angle, and crystal birefringence. Experimental validation conducted on mercurous halide and tellurium dioxide crystals demonstrates that higher birefringence in crystals significantly amplifies the separation angle, augmenting the device's performance. The study contributes to the development of devices with large separation angles during the design phase, enhancing systematic throughput in spectral imaging applications.

Acousto-optic-based time domain electric field sensor for magnetic resonance imaging applications.

An acousto-optic (AO)-based electric field sensor is presented for time domain measurement under magnetic resonance imaging (MRI). A fully MR-compatible sensor is designed and fabricated using a phase-shifted fiber Bragg grating mechanically coupled to a piezoelectric transducer. Mechanical resonance of the piezoelectric transducer is matched to the operating frequencies of commonly used MRI systems to increase the sensitivity of the sensor. Sensitivity of the sensor is measured as 1.27 mV/V/m, with a minimum detectable electric field of 4.4 mV/m/√/Hz. Directivity of the sensor is measured with a 18 dB orthogonal component rejection. The dynamic range of the sensor is calculated as 117 dB/Hz, which allows the measurement of electric fields up to 3.2 kV/m. In MRI studies, the AO sensor was able detect local hot spots around a reference implant accurately with high signal-to-noise ratio. AO sensor exhibited similar or better performance when compared with commercially available MRI compatible electric field sensors. Furthermore, the small size of the sensor with the flexible fiber optic link could allow in situ measurements of electric fields during critical interventional procedures such as pacemaker lead or deep brain stimulator placement as an MRI dosimeter during diagnostic scans.

Investigation of acousto-optic interaction with momentum mismatching considering acoustic anisotropy in birefringent crystal.

In this work, the momentum mismatching based on which the acousto-optic (AO) transfer function and diffraction efficiency was acquired, was calculated considering the properties of AO crystals in AO interactions in acousto-optic tunable filter (AOTF). Transfer functions were obtained using a 4f optical system combined with AOTF and compared with theoretical calculations. It demonstrated the influence of acoustic energy shift on the AO interaction which should be considered in the design of AOTF.

Watt-level LED-pumped actively Q-switched 1319 nm laser with high repetition rate operation

In this paper, we exhibited a watt-level acousto-optical (A-O) Q-switched 1319 nm laser based on a high-efficiency LED-pumped Nd:YAG laser module with high average power and high repetition rate operation. For the quasi-continuous wave (QCW) running operation, the average output power of fundamental laser at 1319 nm was as high as 4.73 W with a pulse length of 972 μs at a repetition rate of 100 Hz. After the resonator structure was optimized by A-O Q-switched modulation, the maximum power was 2.35 W at a repetition frequency of 5 kHz with a pulse width of 1.52 μs, and the M2 factor was measured to be about 9.4. To the best of my knowledge, this is the first demonstration, the maximum average power and high repetition rate watt-level output of an LED-pumped A-O Q-switched 1319 nm laser reported to date.

Silicon-Lattice-Matched Boron-Doped Gallium Phosphide: A Scalable Acousto-Optic Platform.

The compact size, scalability, and strongly confined fields in integrated photonic devices enable new functionalities in photonic networking and information processing, both classical and quantum. Gallium phosphide (GaP) is a promising material for active integrated photonics due to its high refractive index, wide bandgap, strong nonlinear properties, and large acousto-optic figureof merit. This study demonstrates that silicon-lattice-matched boron-doped GaP (BGaP), grown at the 12-inch wafer scale, provides similar functionalities as GaP. BGaP optical resonators exhibit intrinsic quality factors exceeding 25,000 and 200,000 at visible and telecom wavelengths, respectively. It further demonstrates the electromechanical generation of low-loss acoustic waves and an integrated acousto-optic (AO) modulator. High-resolution spatial and compositional mapping, combined with ab initio calculations, indicate two candidates for the excess optical loss in the visible band: the silicon-GaP interface and boron dimers. These results demonstrate the promise of the BGaP material platform for the development of scalable AO technologies at telecom and provide potential pathways toward higher performance at shorterwavelengths.