3He Neutron Spin Filter Research Articles

Micro in situ 3He Polarizer for Dimensional Extreme Magnetic Neutron Diffractometer at the High Flux Isotope Reactor

A new micro in situ polarized 3He neutron spin filter has been custom built for use as a neutron polarizer on the Dimensional Extreme Magnetic Neutron Diffractometer (DEMAND) at the High Flux Isotope Reactor (HFIR). The 3He is polarized via spin-exchange optical pumping with a high-power fiber-coupled laser. The 3He neutron spin filter polarizer is designed to be compact in size with the length along the neutron beam only 30 cm because of the limited space available on the beamline. The polarizer is used for the shorter wavelength neutrons (1.005 Å and 1.546 Å) at DEMAND. A 3 bar 3He cell was filled to provide enough opacity so that good neutron polarization can be attained. At DEMAND the polarizer is mounted on an Automated Polarizer Changeover system (APCS) enabling quick switching between polarized and unpolarized neutron diffraction.

In-situ 3He neutron spin filters at JCNS, status and updates

The JCNS has been developing and using in-situ polarized neutron spin filters for many applications. The system used for analysis on MARIA and polarization for TOPAS were completed about 10 years ago with the MARIA system in standard operation for users and the TOPAS system employed for a long measurement on the POLI instrument. In the meantime we are progressing on several new in-situ polarizers based on these first two but with additional innovations. The KWS-1 analyzer device which was recently used in tests at TU Delft and ISIS is essentially a 50%-sized copy of the MARIA device. The two devices in construction for polarization and analysis on POLI for hot neutrons feature magic-boxes with angled plates on both the entrance and exit sides to minimize overal length and the polarizer device will employ an additional passive magnetic shield of soft iron so that it can operate inside the stray field area of a 8-T vertical (compensated) sample magnet. We will summarize the current status of our 3He neutron spin filters and provide extra focus on the technical aspects and measured performance characteristics of the new devices for KWS-1 and POLI in particular.

Polarisation Development at the European Spallation Source

To meet the ever-increasing user demand, eleven of the fifteen European Spallation Source (ESS) instruments under construction aim to offer polarised neutrons for user experiments. They include an imaging instrument, a SANS instruments, two reflectometers, three diffractometers, and four spectrometers. In conjunction with in-kind contributions and instrumentation grants, the ESS Polarisation Project will support the incorporation of polarisation analysis on eight of the eleven instruments. The project aims to deliver polarised neutrons for first-science experiments as instruments enter operation. Different polariser and polarisation analyser techniques will be available to accommodate the specifics of experiments on a given instrument. Polarised 3He neutron spin filter using either Metastable Optical Pumping (MEOP) or Spin-Exchange Optical Pumping (SEOP) techniques will provide shared-use equipment among many instruments, with SEOP’s main application being in situ beam-polarisation. Several instruments will also use polarising-supermirror devices. To provide wide-bandwidth spin-flipping capability to the time-of-flight instruments, Adiabatic Fast Passage (AFP) neutron spin flippers, also known as gradient-field radiofrequency spin flippers will be the main method of choice. Devices based on the same AFP principle will also be used to flip 3He nuclear spins. We are constructing our first 3He polariser setup, including field coils to produce highly uniform magnetic field. Monte Carlo simulations are being done for the supermirror polarisers. To ensure science-focused development, we are working with university partners in doing scientific experiments with polarised neutrons. These are some of the activities developing polarisation analysis for ESS instruments in our project.

Development of a Spin-Exchange Optical Pumping-Based Polarized 3He System at the China Spallation Neutron Source (CSNS)Supported by the National Key Research and Development Program of China (Grant No. 2020YFA0406000), the National Natural Science Foundation of China (Grant No. 11875265), the Scientific Instrument Developing Project of the Chinese Academy of Sciences (Grant No. 284(2018)), Guangdong Basic and Applied Basic Research Foundation

Polarized 3He neutron spin filters (NSFs) can be used as a vital tool for neutron polarization production and analysis. The China Spallation Neutron Source (CSNS), as one of the major neutron facilities in China, has committed resources to the development of a polarized 3He NSF program to support its growing polarized neutron research. A spin-exchange optical pumping (SEOP)-based polarized 3He system and other necessary hardware for NSF transport has been recently developed. The performance of the system is benchmarked using an in-house developed cell named “Trident”. Neutron beam measurements yield a 3He polarization of 77% with over 200 h of on-beam relaxation time. Combining this newly developed SEOP system with the recently reported cell fabrication station, CSNS is now capable of the fully self-sustained production of 3He NSFs that shall support its future neutron polarization research.

New design of a magnetic device for wide-angle XYZ polarization analysis PASTIS-3, from the concept to first tests with thermal neutrons

We present the new concept and neutron test results of the third generation PASTIS device for XYZ wide-angle polarization analysis for thermal neutrons. PASTIS-3 uses two polarized 3He Neutron Spin filter Cells (NSF) for polarizing and analyzing neutrons spins, flipping the incident neutron beam polarization by reversing the 3He spin state of the polarizing entrance cell. We detail a new coil design for high spatial homogeneity of the magnetic field in any field direction, and the calculation method employed to optimize the geometry and to characterize the field gradients. Various components of the apparatus are described with particular attention to their performance and impact on the relaxation time of the NSF cells. Finally, we present test results of the new device tested on the thermal triple-axis spectrometer IN20 at the ILL.

Optimizing magnetically shielded solenoids.

An important consideration when designing a magnetostatic cavity for various applications is to maximize the ratio of the volume of field homogeneity to the overall size of the cavity. We report a design of a magnetically shielded solenoid that significantly improves the transverse field gradient averaged over a volume of 1000 cm3 by placing compensation coils around the holes in the mu-metal end caps rather than the conventional design in which the compensation coils are placed on the main solenoid. Our application is polarized 3He-based neutron spin filters, and our goal was to minimize the volume-averaged transverse field gradient, thereby the gradient induced relaxation time, over a 3He cell. For solenoids with end cap holes of different sizes, additional improvements in the field gradient were accomplished by introducing non-identical compensation coils centered around the non-identical holes in the end caps. The improved designs have yielded an overall factor of 7 decrease in the gradient in the solenoid, hence a factor of 50 increase in the gradient induced relaxation time of the 3He polarization. The results from both simulation and experiments for the development of several such solenoids are presented. Whereas our focus is on the development of magnetically shielded solenoids for 3He neutron spin filters, the approach can be applied for other applications demanding a high level of field homogeneity over a large volume.

Experimental test of 3He neutron-spin filter in MIEZE spectrometer

A modulated intensity by zero effort (MIEZE) spectrometer is a type of neutron-resonance spin-echo spectrometer and can be used to analyze the slow dynamics of condensed matter by measuring the intermediate scattering function I(Q,τ). A crucial feature of a MIEZE spectrometer is it leaves completely free the space between the sample and the detector because the sample is placed after the neutron-spin analyzer. Measuring the magnetic dynamics with a conventional neutron-spin-echo spectrometer is difficult, but with a MIEZE spectrometer such a measurement may be done simply by introducing a second analyzer after the sample. Measuring the magnetic dynamics with high precision requires the background to be reduced to a minimum and is a job for which a 3He neutron-spin filter (3He-NSF) is a promising candidate as a second analyzer. However, one difficulty with this approach is the diffusion of 3He gas from the 3He-NSF, which may be measured and interpreted as dynamics. Therefore, we investigate herein whether the dynamics of gas diffusion is detected when using a 3He-NSF as second analyzer in a MIEZE spectrometer. Toward this end, we experimented with the MIEZE spectrometer installed at beamline 06 (BL06) at the Materials and Life Science Experimental Facility at Japan Proton Accelerator Research Complex (J-PARC MLF). The results confirm that the gas-diffusion dynamics of the 3He-NSF are not detected, and that the 3He-NSF, therefore, can be used as a second analyzer in this MIEZE spectrometer.

Optimization of a magnetostatic cavity for a 3He spin analyzer on the CANDOR polychromatic reflectometer

A new instrument, the CANDOR (Chromatic Analysis Neutron Diffractometer or Reflectometer) polychromatic beam reflectometer is being built at the National Institute of Standards and Technology Center for Neutron Research. CANDOR will have a capability of polarization analysis for both specular and off-specular scattering, and allow for measuring the magnetic structures of magnetic thin films with a significantly shortened measurement time as compared to a conventional monochromatic beam reflectometer at a continuous neutron source. A critical component of the polarization analysis capability is to develop a 3He neutron spin filter (NSF) for polarization analysis for both specular and off-specular scattering for a continuous wavelength range between 4 Å and 6 Å and a large solid angle coverage for up to 20 energy dispersive detector channels. For ex-situ spin-exchange optical pumping (SEOP) operation, a magnetically shielded solenoid (MSS) will be employed to provide a volume averaged field gradient, better than 5×10−4 cm−1 to maintain 3He polarization relaxation times of at least a few hundred hours on the beam line even when there are significant stray fields from a magnet operating at a field up to 3 T at the sample position. We describe a procedure to design, construct, and optimize a MSS with non-identical compensation coil dimensions on the ends to match the scattered neutron beam rays. The volume averaged field gradient is quantified and optimized over a cell for a MSS using the finite-element software package RADIA and compared with that from the experiment.

In-situ 3He SEOP polarizer for Thermal neutrons

In this article, we describe a neutron polarizer for a new time-of-flight neutron spectrometer with the polarization analysis TOPAS. This instrument will use the convergent focused incoming beam of thermal neutrons with energies up to 150 meV (wavelength down to 0.74Å). The polarizer employs a high opacity 3He neutron spin filter with continuous 3He polarization provided by two laser array bars frequency narrowed by an ultra-compact volume Bragg grating. The system was successfully prototyped, and tested. In the course of first experimental test at the polarized hot neutron diffractometer POLI at MLZ, neutron polarization of 97.6% was achieved for 0.895Å neutrons and kept constant during 30 days.

Generation and detection of spin-orbit coupled neutron beams

Spin-orbit coupling of light has come to the fore in nanooptics and plasmonics, and is a key ingredient of topological photonics and chiral quantum optics. We demonstrate a basic tool for incorporating analogous effects into neutron optics: the generation and detection of neutron beams with coupled spin and orbital angular momentum. The 3He neutron spin filters are used in conjunction with specifically oriented triangular coils to prepare neutron beams with lattices of spin-orbit correlations, as demonstrated by their spin-dependent intensity profiles. These correlations can be tailored to particular applications, such as neutron studies of topological materials.

Development of a polarized 3He neutron spin filter based on spin exchange optical pumping at China Mianyang Research Reactor

Development of a polarized 3He neutron spin filter based on spin exchange optical pumping at China Mianyang Research Reactor

Materials and Life Science Experimental Facility at the Japan Proton Accelerator Research Complex III: Neutron Devices and Computational and Sample Environments

Neutron devices such as neutron detectors, optical devices including supermirror devices and 3He neutron spin filters, and choppers are successfully developed and installed at the Materials Life Science Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC), Tokai, Japan. Four software components of MLF computational environment, instrument control, data acquisition, data analysis, and a database, have been developed and equipped at MLF. MLF also provides a wide variety of sample environment options including high and low temperatures, high magnetic fields, and high pressures. This paper describes the current status of neutron devices, computational and sample environments at MLF.

Discussion on data correction for Polarization Analysis with a 3He spin filter analyzer

Fully polarized neutron reflectometry and grazing incidence small angle neutron scattering are effective methods to explore magnetic structures on the nm to μm length scales. This paper is an outline of how to fully correct for the polarization analysis (PA) inefficiencies of such an instrument and to determine the error contributions of the neutron polarizer and analyzer. This discussion considers the exact case of the polarization analysis instrumentation used on the MARIA neutron reflectometer at the MLZ or for a general polarized neutron scattering instrument using at least one 3He neutron spin filter that has the capability for adiabatic fast passage nuclear magnetic resonance flipping of the 3He polarization. This paper will work to build a conceptual understanding of how the inefficiencies of neutron polarization elements affect measured data in order to stress and encourage the application of PA corrections and to help perform successful measurements. Then, using data from a fully polarized neutron reflectometer test measurement we show how it is possible to recover signals on the order of, or even smaller than, the inefficiencies, or bleed-through, of the neutron polarization devices used.

Development of a polarized 3He neutron spin filter for POLANO at J-PARC

We have developed a polarized 3He neutron spin filter (NSF) for a new polarized neutron spectrometer, POLANO, at the Japan Proton Accelerator Research Complex (J-PARC). POLANO aims to utilize high energy neutrons polarized by a 3He NSF and spin analyzed by an array of magnetic supermirrors for inelastic neutron scattering. The 3He gas is continuously polarized in-situ by spin-exchange optical pumping to provide a highly and stably polarized neutron beam. The POLANO 3He NSF is designed to polarize neutrons with energies as high as 200 meV and fit in a restricted space. It is equipped with adiabatic fast passage NMR that enables one to flip the 3He spins, and consequently, the neutron spins.

Recent on-beam tests of wide angle neutron polarization analysis with a 3He spin filter: Magic PASTIS on V20 at HZB

A complete XYZ polarization analysis solution is under development for the new thermal time of flight spectrometer TOPAS [1], to be operated in the coming east neutron guide hall at the MLZ. Polarization Analysis Studies on a Thermal Inelastic Spectrometer, commonly called PASTIS [2], is based on polarized 3He neutron spin filters and an XYZ field configuration for the sample environment and a polarization-preserving neutron guide field. The complete system was designed to provide adiabatic transport of the neutron polarization to the sample position while maintaining the homogeneity of the XYZ field. This system has now been tested on the polarized time-of-flight ESS test beam line V20 at HZB [3]. Down to the minimum wavelength of 1.6 Å on the instrument, the magnetic configuration worked ideally for neutron spin transport while giving full experimental freedom to change between the X, Y or Z field configuration. The 3He cell used was polarized at the 3He lab of the JCNS at the MLZ in Garching and transported to HZB in Berlin via car showing that such a transport is indeed feasible for such experiments. We present results of this test and the next steps forward.

Development of an in-situ SEOP 3He Neutron Spin Filter for Magnetic Imaging Techniques

We have been developing a 3He neutron spin filter (NSF) using a spin exchange optical pumping (SEOP) technique. The 3He NSF provides a high-energy polarized neutron beam with large beam size. A high-energy polarized neutron beam, which is more difficult to produce with commonly used magnetic supermirror-based polarizers, is an effective probe for magnetic imaging techniques, particularly in the case of strong magnetic fields. Additionally, an in-situ SEOP system enables us to produce a polarized neutron beam with stable polarization, which is big advantage for experiments with long measurement times. In this study, we installed two in-situ SEOP systems as a neutron spin polarizer and analyzer providing a stable high-energy polarized neutron beam over several days.

Recent advancements of wide-angle polarization analysis with 3He neutron spin filters

Wide-angle polarization analysis with polarized 3He based neutron spin filters (NSFs) has recently been employed on the Multi-Axis Crystal Spectrometer (MACS) at the National Institute of Standards and Technology Center for Neutron Research (NCNR). Over the past several years, the apparatus has undergone many upgrades to address the fundamental requirements for wide angle polarization analysis using spin exchange optical pumping based 3He NSFs. In this paper, we report substantial improvements in the on-beam-line performance of the apparatus and progress toward routine user capability. We discuss new standard samples used for 3He NSF characterization and the flipping ratio measurement on MACS. We further discuss the management of stray magnetic fields produced by operation of superconducting magnets on the MACS instrument, which can significantly reduce the 3He polarization relaxation time. Finally, we present the results of recent development of horseshoe-shaped wide angle cells.

Neutron depolarization imaging of the hydrostatic pressure dependence of inhomogeneous ferromagnets

The investigation of fragile and potentially inhomogeneous forms of ferromagnetic order under extreme conditions, such as low temperatures and high pressures, is of central interest for areas such as geophysics, correlated electron systems, as well as the optimization of materials synthesis for applications where particular material properties are required. We report neutron depolarization imaging measurements on the weak ferromagnet Ni3Al under pressures up to 10 kbar using a Cu:Be clamp cell. Using a polychromatic neutron beam with wavelengths λ≥4 Å in combination with 3He neutron spin filter cells as polarizer and analyzer, we were able to track differences of the pressure response in inhomogeneous samples by virtue of high resolution neutron depolarization imaging. This provides spatially resolved and non-destructive access to the pressure dependence of the magnetic properties of inhomogeneous ferromagnetic materials.

Development of a 3He nuclear spin flip system on an in-situ SEOP 3He spin filter and demonstration for a neutron reflectometer and magnetic imaging technique

We have been developing a 3He neutron spin filter (NSF) using the spin exchange optical pumping (SEOP) technique. The 3He NSF provides a high-energy polarized neutron beam with large beam size. Moreover the 3He NSF can work as a π-flipper for a polarized neutron beam by flipping the 3He nuclear spin using a nuclear magnetic resonance (NMR) technique. For NMR with the in-situ SEOP technique, the polarization of the laser must be reversed simultaneously because a non-reversed laser reduces the polarization of the spin-flipped 3He. To change the polarity of the laser, a half-wavelength plate was installed. The rotation angle of the half-wavelength plate was optimized, and a polarization of 97% was obtained for the circularly polarized laser. The 3He polarization reached 70% and was stable over one week. A demonstration of the 3He nuclear spin flip system was performed at the polarized neutron reflectometer SHARAKU (BL17) and NOBORU (BL10) at J-PARC. Off-specular measurement from a magnetic Fe/Cr thin film and magnetic imaging of a magnetic steel sheet were performed at BL17 and BL10, respectively.

Conceptual design of a polarized 3He neutron spin filter for polarized neutron spectrometer POLANO at J-PARC

A 3He neutron spin filter (NSF) has been designed for a new polarized neutron chopper spectrometer called the Polarization Analysis Neutron Spectrometer with Correlation Method (POLANO) at the Materials and Life Science Experimental Facility of the Japan Proton Accelerator Research Complex. It is designed to fit in a limited space on the spectrometer as an initial neutron beam polarizer and is polarized in situ by spin exchange optical pumping. This will be the first generation 3He NSF on POLANO, and a polarized neutron beam up to 100 meV with a diameter of 50 mm will be available for research on magnetism, hydrogen materials, and strongly correlated electron systems.