Abstract
Triphenyleneethynylene (TPE) monolayers at the solution-HOPG interface are oligomerized by the oxidation of pendant thioethers to form disulfide cross-links. The oligomerized TPE monolayer adheres strongly to HOPG. Disulfide reduction unzips the oligomers to form a monomeric TPE monolayer with pendant thiols. Subsequent oxidation and reduction treatments zip and unzip the monolayer.
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