Abstract

Abstract. We developed the WRF-GC model, an online coupling of the Weather Research and Forecasting (WRF) mesoscale meteorological model and the GEOS-Chem atmospheric chemistry model, for regional atmospheric chemistry and air quality modeling. WRF and GEOS-Chem are both open-source community models. WRF-GC offers regional modellers access to the latest GEOS-Chem chemical module, which is state of the science, well documented, traceable, benchmarked, actively developed by a large international user base, and centrally managed by a dedicated support team. At the same time, WRF-GC enables GEOS-Chem users to perform high-resolution forecasts and hindcasts for any region and time of interest. WRF-GC uses unmodified copies of WRF and GEOS-Chem from their respective sources; the coupling structure allows future versions of either one of the two parent models to be integrated into WRF-GC with relative ease. Within WRF-GC, the physical and chemical state variables are managed in distributed memory and translated between WRF and GEOS-Chem by the WRF-GC coupler at runtime. We used the WRF-GC model to simulate surface PM2.5 concentrations over China during 22 to 27 January 2015 and compared the results to surface observations and the outcomes from a GEOS-Chem Classic nested-China simulation. Both models were able to reproduce the observed spatiotemporal variations of regional PM2.5, but the WRF-GC model (r=0.68, bias =29 %) reproduced the observed daily PM2.5 concentrations over eastern China better than the GEOS-Chem Classic model did (r=0.72, bias =55 %). This was because the WRF-GC simulation, nudged with surface and upper-level meteorological observations, was able to better represent the pollution meteorology during the study period. The WRF-GC model is parallelized across computational cores and scales well on massively parallel architectures. In our tests where the two models were similarly configured, the WRF-GC simulation was 3 times more efficient than the GEOS-Chem Classic nested-grid simulation due to the efficient transport algorithm and the Message Passing Interface (MPI)-based parallelization provided by the WRF software framework. WRF-GC v1.0 supports one-way coupling only, using WRF-simulated meteorological fields to drive GEOS-Chem with no chemical feedbacks. The development of two-way coupling capabilities, i.e., the ability to simulate radiative and microphysical feedbacks of chemistry to meteorology, is under way. The WRF-GC model is open source and freely available from http://wrf.geos-chem.org (last access: 10 July 2020).

Highlights

  • Regional models of atmospheric chemistry simulate the emission, transport, chemical evolution, and removal of atmospheric constituents over a given domain

  • We present here the development of a new regional atmospheric chemistry model: WRF-GC, an online coupling of the Weather Research and Forecasting (WRF) mesoscale meteorological model and the GEOS-Chem atmospheric chemistry model, designed to allow easy updates and be computationally efficient, for use in research and operation applications

  • Distributed parallelism is implemented through the Runtime System Library lite (RSL-lite) module, which supports irregular domain decomposition, automatic index translation, distributed input/output, and low-level interfacing with Message Passing Interface (MPI) libraries (Michalakes et al, 1999)

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Summary

Introduction

Regional models of atmospheric chemistry simulate the emission, transport, chemical evolution, and removal of atmospheric constituents over a given domain. GEOS-Chem offers a number of specialty simulations to address a variety of scientific questions, such as simulations of CO2 (Nassar et al, 2010), CO (Fisher et al, 2017), methane (Maasakkers et al, 2019), mercury (Horowitz et al, 2017; Soerensen et al, 2010), persistent organic pollutants (Friedman et al, 2013), and dicarbonyls (Fu et al, 2008, 2009; Cao et al, 2018) Despite their updated representation of chemical processes and relative ease of use, offline models have several key shortcomings. WRF-GC allows GEOS-Chem users to perform highresolution simulations in both forecast and hindcast modes at any location and time of interest The nested domain and two-way coupling capabilities are under development and will be described in a forthcoming paper (Feng et al, 2020)

The WRF model
The GEOS-Chem model
Overview of the WRF-GC model architecture
Further modularization of GEOS-Chem for WRF-GC coupling
Installation and compilation process
Runtime processes
Treatment of key processes in the WRF-GC coupled model
Emission of chemical species
Subgrid vertical transport of chemical species
Dry deposition and wet scavenging of chemical species
Setup of the WRF-GC model and the GEOS-Chem model
Computational performance of the WRF-GC model
Scalability of the WRF-GC model
Findings
Conclusions
Full Text
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