Abstract

As a typical structural energy-containing material, aluminium/polytetrafluoroethylene (Al/PTFE) exhibits excellent mechanical properties under conventional conditions and releases large amounts of energy through chemical reactions under impact loading. In this research, a viscoelastic-damage constitutive model suitable for polymer-based reactive materials was developed, which consisted of an elastic element, two Maxwell elements, and a SCRAM damage element. The effect of damage on the stress–strain relationship was obtained by analysing the crack evolution process and deformation field. A modified Split Hopkinson pressure bar experiment investigated the mechanical characteristics of aluminium/polytetrafluoroethylene under uniaxial/multiaxial impact loading. The results indicated that the viscoelastic-damage constitutive model could describe the effects of the initial crack size and initial crack density on the mechanical properties of aluminium/polytetrafluoroethylene. With the decrease in initial crack length and density, the damage to the aluminium/polytetrafluoroethylene under impact loading was limited, which caused the dynamic mechanical properties to increase. When the pre-stress increases from 0 MPa to 10 MPa, the dynamic ultimate compressive stress of aluminium/polytetrafluoroethylene increases from 77.2 MPa to 89.8 MPa at 2910 s−1 strain rate. A comparison of the experimental and calculated strain–stress curves shows that the established constitutive model is feasible to predicting the mechanical behaviour of aluminium/polytetrafluoroethylene.

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