Abstract
Vinylcyclopropyl substituted diazenes (e.g. 1 and 15 ) rearrange when heated. The chemistry takes place via the formation of a trimethylenemethane (TMM) diyl and provides access to eight-membered rings. When the cyclopropane is fused to a five-membered ring (e.g. 15 ) rearrangement leads to a structure resembling the taxotere framework.
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