Abstract
FT-IR and Raman spectra of S-methyl-N,N-dimethylmonothiocarbamate and its d 3-, d 6-, d 9-, and 13C-substituted isotopomers have been recorded and analysed. Normal coordinate calculations were performed to support the assignment and to derive a simplified valence force field which would be characteristic of the monothiocarbamate moiety, =N(CO)S-, and is consistent with the known bond length vs force constant correlations.
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