Abstract
The vibrational relaxation of laser excited O3(001) by H2O and D2O has been studied over the temperature range 295–473 °K. The CO2 laser-induced chemiluminescent reaction of NO+O3(001) was utilized to monitor the decay rate of vibrationally excited ozone. The relaxation probability for both water isotopes has a strong inverse temperature dependence, with D2O being four times more efficient than H2O. The results are discussed in terms of a metastable complex model for energy transfer.
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