Abstract
The theory of computing mean-square parallel and perpendicular amplitudes from spectroscopic data, developed by Morino and Hirota, is summarized. A slightly modified method is proposed, connecting these quantities to the concept of mean-square amplitude matrices. As a particular case, the tetrahedral XY 4 molecular model is considered, and all the nonvanishing generalized mean-square amplitudes for the bonded and nonbonded distance types are given. The quantities are expressed as linear combinations of the symmetrized mean-square amplitude matrfix.
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