Abstract
Vibrational fluorescence from the V = 2 to the V = 1 state is observed following excitation by a pulsed HBr chemical laser. The time dependence of the fluorescence is used to determine the rate of near-resonant vibration-to-vibration energy transfer, HBr( V = 1) + HBr( V = 1) ⇌ HBr( V = 2) + HBr( V = 0) + δ E = 90 cm −1. The cross section for this reacti
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