Abstract
Abstract Vibrational correlation functions obtained from the isotropic Raman scattering of the P—H stretching vibration of PHD 2 isolated as an isotopic impurity in liquid and solid PD 3 have been modeled using a memory-function appraoch. The modulation is fast all temperatures. It is postulated that rotation—translation coupling is responsible for the vibrational relaxation. Information about the molecular dynamics has been obtained out to 7 ps.
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