Abstract
Vibrational absorption bands of methyl isocyanide and its d3-derivative have been measured with higher resolution than previously, and the rotational structure of some bands has been analysed. The band origins have been determined for some parallel bands and molecular constants have been derived. A more detailed examination of the fundamental bands of the degenerate vibrations of both molecules has led to a determination ofA"and of the Coriolis coupling coefficients forv5,v6,v7andv8. Several perturbations arising from Fermi or Coriolis interactions have been explained.
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More From: Proceedings of the Royal Society of London. A. Mathematical and Physical Sciences
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