Abstract
Excited states in 212,213Rn were populated in the bombardment of 204Hg by 14C ions of energies 80-94 MeV. The depopulation of the excited states was studied using in-beam spectroscopic methods including γ-ray excitation, γ-ray angular distribution, γ-γ-t coincidence, pulsed-beam-γ timing and conversion electron measurements. Spins up to Jπ = 30ℏ and a tentative J = (73/2)ℏ were observed, respectively. In 212Rn the previous level scheme was confirmed, with the addition of five new transitions of which one feeds the 30+ state. In 213Rn the previously reported level scheme was mainly confirmed and it was extended to (71/2) or (73/2)ℏ, which is the highest spin observed to-date in a lead-region nucleus. Several transition rates B(λ) were deduced from isomeric half-lives or branching ratios in both isotopes. Deformed Independent Particle Model (DIPM) calculations were performed to assign configurations, which in 213Rn usually consist of the odd neutrons vg9/2 and vj15/2 coupled to the four-proton states in 212Rn. The highest levels include neutron core-excitations, since the maximum valence-nucleon angular momentum in 213Rn is 55/2ℏ. The very topmost levels even need 2- particle-two-hole excitations. Shape changes in these two Rn isotopes are discussed, as are the transition rates.
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