Abstract

Ground-state and excited-state properties of vertically coupled double quantum dots are studied by exact diagonalization. Magic-number total angular momenta that minimize the total energy are found to reflect a crossover between electron configurations dominated by intra-layer correlation and ones dominated by inter-layer correlation. The position of the crossover is governed by the strength of the inter-layer electron tunneling and magnetic field. The magic numbers should have an observable effect on the far infra-red optical absorption spectrum, since Kohn's theorem does not hold when the confinement potential is different for two dots. This is indeed confirmed here from a numerical calculation that includes Landau level mixing. Our results take full account of the effect of spin degrees of freedom. A key feature is that the total spin, $S$, of the system and the magic-number angular momentum are intimately linked because of strong electron correlation. Thus $S$ jumps hand in hand with the total angular momentum as the magnetic field is varied. One important consequence of this is that the spin blockade (an inhibition of single-electron tunneling) should occur in some magnetic field regions because of a spin selection rule. Owing to the flexibility arising from the presence of both intra-layer and inter-layer correlations, the spin blockade is easier to realize in double dots than in single dots.

Highlights

  • Coupled quantum dots have recently attracted much interest, since they open up the possibility of manipulating electron configurations in a threedimensional space

  • Numerical studies of few electron systems confined in single quantum dots have shown that the angular momentum and spin of the ground state in strong magnetic fields belong to a special series values called magic numbers

  • If we plot the position and intensity of the peaks in the far infrared (FIR) spectra along with the ground state total angular momentum L and spin S (Figs. 10 and 11), we find a one-to-one correspondence between the magnetic fields at which the absorption line jumps and the magnetic fields at which the total angular momentum and/or the total spin of the ground state changes from one magicnumber state to another

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Summary

INTRODUCTION

Coupled quantum dots have recently attracted much interest, since they open up the possibility of manipulating electron configurations in a threedimensional space. Ashoori et al and Wagner et al have looked at the addition spectrum (energies required for adding one additional electron) for single dots in magnetic fields, where a total-spin transition caused by the Coulomb interaction is expected [5,6,7] This reminds us of the fractional quantum Hall effect (FQHE) in the bulk 2D electron system, a manifestation of strong electron correlation in high magnetic fields [8,9,10], where the total spin is a sensitive function of the density of electrons in the Landau levels. The wild change in the spin can cause single-electron tunneling to be blocked in some magnetic field regimes due to spin selection rules as we have proposed recently [19] Evidence that this effect is caused by electron correlation is the occurrence of a re-entrant non-blocked region which is hard to explain by Zeeman-energy considerations.

VERTICALLY COUPLED QUANTUM DOTS
MAGIC-NUMBER STATES
Three-electron double dots
Four-electron double dots
Crossover between intra- and inter-layer correlations
Effect of the pseudo-spin Zeeman energy
FIR ABSORPTION
SPIN BLOCKADE
CONCLUSION
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