Abstract

Abstract. This study investigates the vertical transport of a passive tracer in a shallow cumulus boundary layer using large eddy simulations. The tracer source is at the surface in one case, and in the inversion layer in the other case. Results show that shallow cumulus clouds can significantly enhance vertical transport of the tracer in both cases. In the case with surface-borne pollutants, cloudy regions are responsible for the upward transport, due to the intense updrafts in cumulus clouds. In the case where pollutants are aloft, cloud-free regions are responsible for the downward transport, but the downward transport mainly occurs in thin regions around cloud edges. This is consistent with previous aircraft measurements of downdrafts around cumulus clouds and indicates that the downward transport is also cloud-induced. Cumulus convection is therefore able to both vent pollutants upward from the surface and fumigate pollutants in the inversion layer downward into the lower boundary layer.

Highlights

  • Apart from affecting the vertical structure of tropospheric radiative heat flux divergence, and modulating hydrologic cycle, convective clouds can enhance the vertical mixing of gaseous matter and aerosol

  • A passive tracer is used in large eddy simulations for studying the vertical transport of pollutants by shallow cumuli

  • The tracer source is continuous for 4 h at the surface in one case, and is instant in the inversion layer in the other case to investigate both the upward and downward transport associated with cumulus clouds

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Summary

Introduction

Apart from affecting the vertical structure of tropospheric radiative heat flux divergence, and modulating hydrologic cycle, convective clouds can enhance the vertical mixing of gaseous matter and aerosol. More recent studies proposed a refined view of vertical mass transport by cumulus that downdrafts outside clouds are confined in thin shell regions around cloud edges, and that the subsiding shell is attributed to evaporative cooling (Heus and Jonker, 2008; Heus et al, 2009; Jonker et al, 2008) This result can explain the finding that pollutants in the environment far away from cumulus clouds mix very slowly throughout the cloud layer (Verzijlbergh et al, 2009). Yin et al (2005) found that deep convective clouds can transport aerosols from the boundary layer, detrain and re-entrain the aerosols into the middle levels of clouds This process contributes to a large fraction of the aerosols inside hydrometeors (∼ 40 % by mass).

Model and case descriptions
Case 1: vertical transport of pollutants from the surface
Case 2: vertical transport of pollutants from the inversion layer
Conclusions
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