Abstract

Since the COVID-19 outbreak in 2020, China’s air pollution has been significantly affected by control measures on industrial production and human activities. In this study, we analyzed the temporal variations of NO2 concentrations during the COVID-19 lockdown and post-epidemic era in 11 Chinese megacities by using satellite and ground-based remote sensing as well as in situ measurements. The average satellite tropospheric vertical column density (TVCD) of NO2 by TROPOMI decreased by 39.2–71.93% during the 15 days after Chinese New Year when the lockdown was at its most rigorous compared to that of 2019, while the in situ NO2 concentration measured by China National Environmental Monitoring Centre (CNEMC) decreased by 42.53–69.81% for these cities. Such differences between both measurements were further investigated by using ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) remote sensing of NO2 vertical profiles. For instance, in Beijing, MAX-DOAS NO2 showed a decrease of 14.19% (versus 18.63% by in situ) at the ground surface, and 36.24% (versus 36.25% by satellite) for the total tropospheric column. Thus, vertical discrepancies of atmospheric NO2 can largely explain the differences between satellite and in situ NO2 variations. In the post-epidemic era of 2021, satellite NO2 TVCD and in situ NO2 concentrations decreased by 10.42–64.96% and 1.05–34.99% compared to 2019, respectively, possibly related to the reduction of the transportation industry. This study reveals the changes of China’s urban NO2 pollution in the post-epidemic era and indicates that COVID-19 had a profound impact on human social activities and industrial production.

Highlights

  • Atmospheric nitrogen dioxide (NO2 ) is an important atmospheric pollutant

  • The improved TROPOspheric Monitoring Instrument (TROPOMI) NO2 tropospheric vertical column density (TVCD) product by the University of Science and Technology of China (USTC) in this study showed a lower bias in the Chinese region, allowing for more accurate trend analysis [26]

  • It has been demonstrated that the NO2 TVCD obtained from satellite remote sensing observations and NO2 concentrations derived from ground-based stations are consistent, which may be due to their similar sources [39]

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Summary

Introduction

Atmospheric nitrogen dioxide (NO2 ) is an important atmospheric pollutant. NO2 has a significant impact on human health [1,2]. NO2 plays an important role in the formation of ozone and secondary aerosols. 2022, 14, 419 source of tropospheric NO2 concentration [3], which is generally higher near cities. China is one of the most polluted countries in the world in terms of air pollution [4]. With the implementation of new emission regulations in 2011, the NO2 concentrations in China have rapidly decreased as seen from the long-term satellite and ground-based measurements [5,6,7,8]

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