Abstract
Variable fluxes of anthropogenic CO2 emissions into the land and the ocean and the remaining proportion in the atmosphere reflect on the global carbon budget variations and further modulate global climate change. A more accurate reconstruction of the global carbon budget in the past decades and a more reliable prediction of the variations in the next years are crucial for assessing the effectiveness of climate change mitigation policies and supporting global carbon stocktaking and monitoring in compliance with the goals of the Paris Agreement.In this study, we investigate reconstructions and predictions of the CO2 fluxes and atmospheric CO2 growth from ensemble prediction simulations using 5 Earth System Model (ESM) - based decadal prediction systems. These novel prediction systems driven by CO2 emissions with an interactive carbon cycle enable prognostic atmospheric CO2 and represent atmospheric CO2 growth variations in response to the strength of CO2 fluxes into the ocean and the land, which are missing in the conventional concentration-driven decadal prediction systems with prescribed atmospheric CO2 concentration.The reconstructions generated by assimilating physical ocean and atmosphere data products into the prediction systems are able to reproduce the annual mean historical variations of the CO2 fluxes and atmospheric CO2 growth. Multi-model ensemble means best match the assessments of CO2 fluxes and atmospheric CO2 growth rate from the Global Carbon Project with correlations of 0.79, 0.82, and 0.98 for atmospheric CO2 growth rate, air-land CO2 fluxes, and air-sea CO2 fluxes, respectively. The CO2 emission-driven prediction systems with an interactive carbon cycle still maintain the predictive skill of CO2 fluxes and atmospheric CO2 growth as found in conventional concentration-driven prediction systems, i.e., about 2 years for the air-land CO2 fluxes and atmospheric CO2 growth, the air-sea CO2 fluxes have higher skill up to 5 years. The ESM-based prediction systems are capable to reconstruct and predict the variations in the global carbon cycle and hence are powerful tools for supporting carbon budgeting and monitoring, especially in the decarbonization processes. Furthermore, we investigate the contribution of uncertainty in the predictions of CO2 fluxes and atmospheric CO2 growth rate from internal climate variability, different model responses, and emission-forcing reductions to identify the prominent challenge in limiting the skill of CO2 predictions. 
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