Validation Studies of a Computational Model for Molten Material Freezing

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Validation studies are described of a computational model for the freezing of molten core materials under core disruptive accident conditions of fast breeder reactors. A series of out-of-pile experiments named SIMBATH, performed at Forschungszentrum Karlsruhe in Germany, has already been analyzed with the SIMMER-II code. In the current study, TRAN simulation tests in the SIMBATH facility are analyzed by SIMMER-II for its modeling validation of molten material freezing. The original TRAN experiments were performed at Sandia National Laboratories to examine the freezing behavior of molten UO2 injected into an annular channel. In the TRAN simulation experiments of the SIMBATH series, similar freezing phenomena are investigated for molten thermite, a mixture of Al2O3 and iron, instead of UO2.Two typical TRAN simulation tests are analyzed that aim at clarification of the applicability of the code to the freezing process during the experiments. The distribution of molten materials that are deposited in the test section according to the experimental measurements and in calculations by SIMMER-II is compared. These studies confirm that the conduction-limited freezing model combined with the rudimentary bulk freezing (particle-jamming) model of SIMMER-II could be used to reproduce the TRAN simulation experiments satisfactorily. This finding encourages the extrapolation of the results of previous validation research for SIMMER-II based on other SIMBATH tests to reactor case analyses. The calculations by SIMMER-II suggest that further improvements of the model, such as freezing on a convex surface of pin cladding and the scraping of crusts, make possible more accurate simulation of freezing phenomena.