Abstract
The mass and light absorption contributions of organic carbon (OC), elemental carbon (EC), and mineral dust influence glacial melting and potentially contribute to climate change over the high Himalayas and Tibetan Plateau (HTP). Plateau-scale investigations of these components and their respective light absorption are limited due to the high altitude. In this study, we combined the analysis of major light-absorbing substances and their corresponding multiwavelength absorption to determine their specific contributions firstly. We investigated the spatial variations of total suspended particle (TSP) mass across the HTP, noting high contributions from dust, carbonaceous components, and secondary inorganic aerosols (SNA, including sulfate, nitrate, and ammonium). Enhanced levels of primary and secondary OC and SNA were observed in the marginal areas of the HTP, associated with high relative humidity (RH) and OX levels (O3+NO2). EC was the primary contributor to light absorption, accounting for approximately 68%, 46%, and 64% in Ngari, Qinghai Lake, and Beiluhe, respectively. We found higher light-absorbing contributions from carbonaceous aerosols in the marginal areas compared to the central HTP site, particularly during the heating seasons (∼90%). Fugitive dust significantly contributed to TSP mass but not to light absorption. The concurrent constraints on the mass and optical properties of OC, EC, and dust in this study can help reduce uncertainties in climate models specific to the HTP.
Published Version
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