Abstract

A spectroscopic system for the millimeter-wave region has been constructed on the coherent radiation beamline at the KURRI-LINAC of the research reactor institute, Kyoto University. Coherent transition radiation has been used as the light source. The observed spectrum of radiation was distributed throughout the entire millimeter-wave region and the intensity was four orders of magnitude larger than that of the conventional light source which has the continuous spectrum, i.e., a mercury-arc lamp. The interference between wave packets emitted from successive bunches was observed. It showed that the spectrum of coherent transition radiation was constituted of the higher harmonics of the L-band radio frequency (1.3 GHz) and that the high resolution spectrum was not a continuous spectrum. The diameter of the light beam at the position of a sample was about 9 mm (full width half maximum) and it increased as the wavelength became long because of the diffraction effect for the finite sizes of the optical components. Using the spectroscopic system, the pure rotational spectrum of N2O gas was observed in the millimeter-wave region.

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