Using multiple isotopes to determine groundwater source, age, and renewal rate in the Beishan preselected area for geological disposal of high-level radioactive waste in China

Abstract

Understanding hydrogeological conditions is crucial for selecting and assessing the long-term safety performance of a high-level radioactive waste (HLW) disposal repository. Utilizing environmental isotopes as effective markers for analysing groundwater movement, this study investigates groundwater recharge sources, age, and renewal rates using multiple isotopes in China's potential HLW repository site, the Beishan area. The results indicated deep bedrock groundwater primarily derives from ancient precipitation infiltration under cold climatic conditions. A noteworthy distinction is that loose sedimentary groundwater exhibits higher tritium content (>10 TU) compared to bedrock groundwater (<3.2 TU). Groundwater within the recharge area, especially within gullies and piedmont slope deposits, is relatively youthful, with an age of less than 30 years and an annual renewal rate exceeding 5 %. In contrast, the shallow groundwater age in the intermountain basins and depressions of the discharge area generally exceeds 50 years, with an annual renewal rate often falling below 0.5 %. At the Beishan underground research laboratory site, deep groundwater at the disposal repository depth displays a corrected 14C age exceeding 8,000 years, indicating an extremely slow movement and alteration rate. As a result, the hydrogeological conditions in the Beishan area are expected to be relatively beneficial for ensuring the safety of HLW repository.