Abstract

While surface area is one of the most important atmospheric aerosol properties in health effects, methods for online measurement of surface area are not widely available and/or require complex operations. In this paper, we describe an integrated measurement method that can continuously monitor the total surface area, as well as the total number and volume, of atmospheric aerosols. Three integral aerosol sensors - (i) a condensation particle counter (CPC) for number concentration measurement, (ii) a mass concentration monitor (MCM) for mass concentration measurement, and (iii) an electrical aerosol detector (EAD) for current measurement of charged aerosol - are used in this study. Signals from the three sensors are converted into a lognormal size distribution by minimizing the difference between the measured signals and the theoretical values based upon a size distribution model, the instrument calibration, and its theoretical responses. Results from a 20 day continuous sampling period show that the calcul...

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