Unraveling Venus's Atmospheric Composition: Insights into CO, H2O, and OCS Abundances through Observations and Modeling

Abstract

The investigation into Venus's atmosphere has highlighted deficiencies in photochemical models when it comes to explaining the distribution of trace gas species, particularly crucial elements like CO and OCS, which play a vital role in Venus's sulfur cycle and cloud formation. To gain a comprehensive understanding of the abundance and variability of these trace gases ahead of the DaVinci probe's descent, we initiated an observational study using NASA's IRTF telescope equipped with the high-resolution ISHELL spectrometer. Conducted from June 11 to June 30, 2023, our study involved capturing K, H, and J-band spectra of Venus's night side. We employed the SMART software to calculate synthetic spectra, considering various gas abundances and emission angles. With our high-resolution spectral data (R=λ/Δλ~25,000), we successfully mapped the abundances of CO, H2O, and OCS in the equatorial region, revealing both daily and latitudinal variations. Our focus was on examining the delicate balance between chemistry and transport, evident in the observed anti-correlation between OCS and CO abundance with cloud opacity. Through near-infrared observations, this study aims to unravel the intricate interplay between atmospheric dynamics and chemical reactions in Venus's cloud formation. By providing insights into observed cloud patterns and elucidating the relationship between atmospheric chemistry, dynamics, and cloud creation on Venus, we contribute crucial parameters to refine existing photochemical models.