Abstract
Spectral lineshapes of benzene/cyclohexane clusters (B·C N-1 , N=2–20) have been obtained by resonant two-photon ionization spectroscopy in the vicinity of the benzene A 1g→B 2u 6 0 1 transition. An analysis of spectral shifts and multiplicities provides support for the structural shell-filling model used previously to account for (benzene) N cluster spectra. In particular, evidence for isomeric forms of the B·C 6 cluster is interpreted in terms of axial and equatorial sites in the pentagonal bipyramid structure.
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