Ultra-narrowband circular dichroism in all-dielectric chiral nanohole arrays based on griddings and monolayer MoS2

Abstract

The strong circular dichroism (CD) of metallic chiral nanostructures can be applied to polarization conversion, negative refraction materials, and chiral molecule detection. However, metallic chiral nanostructures with losses struggle to produce dynamically tunable ultra-narrow band circular dichroism signals, which greatly limits their applications in sensing. In this paper, the MoS2 and Sb2S3 with phase change characteristics are introduced into all-dielectric chiral nanopore arrays (ACNAs) based on gridding to generate dynamically tunable ultra-narrow band circular dichroism signals. Simulation results show that ACNAs/MoS2 produce two strong narrow-band CD signals in the visible range. The maximum CD intensity can reach 0.75, and the maximum half-width can reach 0.8 nm. The electric field distribution indicates that two CD signals are mainly caused by the guided mode resonance. The ultra-narrow band CD signals both lie on their geometric parameters and can realize the dynamic regulation by changing the incidence angle of lights and the crystalline state of Sb2S3. Furthermore, the sensing characteristics of this device were evaluated by analyzing the effects of different concentrations of SARS-CoV-2 solutions on the CD spectra. These findings will facilitate the design of all-dielectric chiral nanostructures with dynamically tunable ultra-narrow band CDs and facilitate their applications in biosensing.