Abstract

Ultrafast fluorescence spectroscopy has been used to study the solvent mediated excited state intramolecular electron (charge) transfer of 9,9’—bianthryl. The excited state electron transfer (et) kinetics are well modeled by an electronically adiabatic approach, employing an “outer sphere” generalized Langevin equation description of motion along the et reaction coordinate. The relationship between solvation and electron transfer dynamics is discussed.

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