Abstract
Synopsis(X-ray) free-electron lasers are employed to site specifically interrogate atomic fragments during ultra-fast photolysis of chiral molecules via time-resolved photoelectron circular dichroism.
Highlights
To cite this article: P Schmidt et al 2020 J
Ultrafast Structural Changes in Chiral Molecules Measured with FreeElectron Lasers
This has been demonstrated for vibrational excitations[3], multiphoton interactions[4] and ultrafast structural changes[5]. Such exceptional sensitivity of photoelectron circular dichroism (PECD) opens unique perspectives for addressing nonlinear and ultrafast phenomena with VUV and X-ray free-electron lasers that can uniquely enable site selective interrogation of an observing atomic site. Such pump-probe experiments on chiral systems are challenging in terms of their technical, physical andchemical complexity
Summary
Ultrafast Structural Changes in Chiral Molecules Measured with FreeElectron Lasers To cite this article: P Schmidt et al 2020 J. 1 University of Kassel, Institut fur Physik, Heinrich-Plett-Straße 40, 34132
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