Abstract
We experimentally demonstrate N^+_2 lasing actions at the wavelengths of 353.3, 353.8, and 354.9 nm using a circularly polarized femtosecond laser. The three laser lines correspond to the B2Σ+u(v'=5, 4, 3)->X2Σ+g(v'=4,3,2) transitions, respectively. Particularly, we reveal the pressure-dependent gain dynamics of these lasing actions from highly excited vibrational states with a pump–probe scheme. Our experimental results confirm that electron collisional excitation plays an important role in the establishment of a population inversion of N+2 lasing at these wavelengths.
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