Abstract

The recent observation of superconductivity at relatively high temperatures in hole doped NdNiO$_2$ has generated considerable interest, particularly due to its similarity with the infinite layer cuprates. Building on the observation that the Ni$^{2+}$ ions resulting from hole doping are commonly found in the spin-triplet state, we introduce and study a variant of the $t-J$ model in which the holes carry S=1. We name this new model the Type II $t-J$ model. We find two distinct mechanisms for $d$ wave superconductivity. In both scenarios the pairing is driven by the spin coupling $J$. However, coherence is gained in distinct ways in these two scenarios. In the first case, the spin-one holes condense leading to a $d$ wave superconductor along with spin-symmetry breaking. Different orders including spin-nematic orders are possible. This scenario is captured by a spin one slave boson theory. In the second scenario, a coherent and symmetric $d$ wave superconductor is achieved from "Kondo resonance": spin one holes contribute two electrons to form large Fermi surface together with the spin 1/2 singly occupied sites. The large Fermi surface then undergoes $d$ wave pairing because of spin coupling $J$, similar to heavy fermion superconductor. We propose a three-fermion parton theory to treat these two different scenarios in one unified framework and calculate its doping phase diagram within a self consistent mean field approximation. Our study shows that a combination of "cuprate physics" and "heavy fermion physics" may emerge in the type II $t-J$ model.

Highlights

  • A tour de force materials synthesis effort created a thin film of the hole-doped infinite-layer nickelate NdNiO2 [1]

  • According to LDA + U calculations [2,3,4,5,6,7,8,9,10,11], the band at Fermi level is dominated by the dx2−y2 orbital of Ni, which suggests that the main physics may be governed by a one-band Hubbard model as in the cuprates

  • In a certain sense the physics can be understood in the following intuitive way: the doped hole enters the dz2 orbital and forms a small pocket while there is a local spin-1/2 moment sitting on dx2−y2 orbital at every site

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Summary

INTRODUCTION

A tour de force materials synthesis effort created a thin film of the hole-doped infinite-layer nickelate NdNiO2 [1]. In the absence of a direct experimental measurement of the spin state of the doped hole, one cannot rule out the possibility that Ni2+ is in the low-spin state because of a larger energy splitting of the two eg orbitals Such a low spin configuration was proposed in a different but related compound [16] based on certain spectroscopic measurements, more data may be needed to confirm the conclusion. In this case one must revert to a cupratelike t-J model [14,17,18,19,20], at least as far as doped holes are concerned. Doping electrons into the 3d7 configuration is promising in this regard

TYPE-II t-J MODEL
SLAVE BOSON THEORY
THREE-FERMION PARTON THEORY
ROLE OF Nd ORBITAL
CONCLUSION
Distinction from cuprates
Fully Higgsed
Full Text
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