Abstract
Reaction of uranyl nitrate with formic acid in the presence of DABCO or NMe4OH under hydrothermal conditions gave two novel uranyl-organic frameworks. When templated by H-DABCO+ counter-ions, uranyl formate crystallizes as ribbons including μ3-oxo and μ2- and μ3-hydroxo ions. In one experiment with NMe4OH, a nanotubular material was obtained instead of the more usual two- or three-dimensional uranyl formates, with an inner tubule diameter of ca. 6Å.
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