Abstract
NO is a deadly pollutant that makes up more than 90% NOx in a flue gas. NO is insoluble in water; thus, its removal is extremely difficult using the SCR method. This study investigates the feasibility of NO removal and energy efficiency from a coal-combustion flue gas connected to a DBD reactor merged with urea. The results showed that the combined effect of urea and the DBD reactor gave a significant increase in the removal of NO. Comparing the removal efficiencies of NO at different urea mass percentages (9%, 17%, 23%, 29%, and 33%), it was found that the optimum concentration of urea for efficient NO removal was 23% because there is enough NH3 produced at this concentration and less H2O species generated to consume N• free radicals by OH to produce more NO in the system. The removal efficiencies of the optimum 23% urea concentration with oxygen [(NO/N2/O2/CO(NH2)2:23% w/w system] and without oxygen [(NO/N2/CO(NH2)2:23% w/w system] were also compared. It was also found that the addition of urea solution showed a considerably good energy efficiency which implies that the cost of this technology will be effective. The study complements past studies on the efficient removal of NO from the environment.
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