Abstract
Photon scanning tunneling microscopy and spectroscopy using femtosecond two-photon excitation are demonstrated. The measurement of both intensity dependence and spectral dependence is performed on a two-photon chromophore. A subdiffraction-limited resolution is obtained, and the domain-size dependence of spatial and spectral features is observed, which indicates the high degree of molecular order in the isolated nanoparticle. It is shown that the light confinement due to a quadratic dependence of the fluorescence intensity leads to an optical contrast enhancement with a coated probe.
Sign-in/Register to access full text options 
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
