Abstract
We demonstrate that a dipole-dipole interaction of benzo[c][1,2,5]thiadiazole moieties, directional H-bond formation of carboxy groups, and a rigid molecular skeleton enable a structurally-predictable two-dimensional hydrogen-bonded organic framework BTIA-1 from tetratopic carboxylic acid. Activated form BTIA-1a was revealed to have BET surface area of 237 m2g−1 and show selective adsorption of CO2.
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