Abstract
Two hexanuclear complexes of formula [FeIII(Tp*)(CN)3]4[FeII(tptz)]2 (1), [FeIII(Tp*)(CN)3]4[CoII(tptz)]2 (2) [Tp*=hydridotris(3,5-dimethylpyrazolyl)borate, tptz=(2,4,6-tris-(2-pyridyl)1,3,5-triazine] have been synthesized via directional assembly of metallocyanate precursor and metal cationic ions. The magnetic properties characterization indicate that ferromagnetic interactions dominate in the two complexes, resulting in a spin ground state of S=5 and S=6, respectively.
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