Tunnel measurements reveal significant reduction in traffic-related light-absorbing aerosol emissions in China

Abstract

Light-absorbing aerosols (LAA), including black carbon (BC) and brown carbon (BrC), profoundly impact regional and global climate. Vehicle emission is an important source of LAA in urban areas, but real-world emission features of LAA from the urban vehicle fleet are not fully understood. This study evaluates traffic-related BC and BrC emission factors (EFs) and their vehicular emission inventories via road tunnel measurements in Tianjin, China, in 2017 and 2021. The distance-based and fuel-based EFs of BC for the mixed fleet were 1.05 ± 1.28 mg km−1 veh−1 and 0.057 ± 0.057 g (kg-fuel)−1, respectively, in 2021, with a dramatic decrease of 80.6 % compared to those in 2017. The BC EFs for gasoline vehicles (GVs, including traditional gasoline and hybrid vehicles) and diesel vehicles (DVs) were 0.55 ± 0.065 mg km−1 veh−1 and 10.5 ± 2.52 mg km−1 veh−1, respectively, in 2021. Compared to 2017, the BrC EFs also decreased significantly in 2021, by 10.8–53.6 %, with 0.32 ± 0.45 mg km−1 veh−1 and 0.018 ± 0.020 g (kg-fuel)−1 of distance-based and fuel-based EFs for mixed fleet. The BrC EFs for GVs and DVs were 0.091 ± 0.024 mg km−1 veh−1 and 3.06 ± 0.91 mg km−1 veh−1, respectively, in 2021. Based on the BC and BrC EFs for GVs and DVs and annual mileage for each vehicle category, the annual vehicular LAA emission inventories were estimated. From 2017 to 2021, the annual vehicular LAA emissions in Tianjin have been significantly reduced, by 69 % for BC and 10 % for BrC. DVs account for a small amount of the vehicle population (8.4 %), but contribute to most of the BC (83 %) and BrC (86 %). Our study demonstrates the significant reduction of vehicular light-absorbing aerosols emission due to vehicle pollution prevention and control in China.