Tuning in-plane and out-of-plane exchange biases in Ni80Fe20/Cr-oxide bilayers

Abstract

The exchange bias effects of NiFe/Cr-oxide bilayers were studied. Results have shown that NiFe/Cr-oxide bilayers exhibited an exchange bias loop shift when field cooled to 5 K. A strong linear dependence of ferromagnetic NiFe and antiferromagnetic Cr2O3 thicknesses on the exchange bias field Hex was observed. The largest interfacial exchange energy Eint∼5.4×10−2 erg/cm2 was found in bilayers with the thickest Cr2O3 layer indicating that stronger interface exchange coupling is enabled by thicker Cr2O3 layers. In addition, Hex decreased linearly with increasing %O2/Ar ratio, reflecting that ion-beam bombardment tends to degrade the Cr2O3 surface spin structures. We also find that annealing the Cr-oxide layer yields both a structural phase transformation and improved crystallinity, giving rise to stronger exchange bias behavior. Further, the coexistence of in-plane as well as out-of-plane exchange biases was observed in a NiFe/annealed Cr2O3/Al2O3(0001) bilayer. This clearly indicates that by using the single crystal Al2O3(0001) substrate together with a rapid thermal annealing process, the antiferromagnet Cr2O3 spins are tilted toward the out-of-plane direction and thus exhibit this unusual exchange bias behavior.