Abstract

A solid-state organic thin-film laser with intracavity frequency doubling is reported. Tunable ultraviolet emission from 309 to 322 nm is achieved from a vertical external cavity surface-emitting organic laser, with 2% efficiency (1 μJ at 315 nm). The laser comprises a poly(methyl methacrylate) layer doped with Rhodamine 640, spun-cast onto a plane mirror, a remote concave mirror, a nonlinear crystal, and a dichroic separator. The output is spectrally narrow (<0.5 nm full width at half maximum) and tunable through phase-matching selection of the fundamental radiation lasing modes. These results highlight a low-cost and portable alternative to tunable UV laser sources, useful for spectroscopic applications.

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