Abstract

We present a solid-state laser system that generates over 200 mW of continuous-wave, narrowband light, tunable from 316.3 nm - 317.7 nm and 318.0 nm - 319.3 nm. The laser is based on commercially available fiber amplifiers and optical frequency doubling technology, along with sum frequency generation in a periodically poled stoichiometric lithium tantalate crystal. The laser frequency is stabilized to an atomic-referenced high finesse optical transfer cavity. Using a GPS-referenced optical frequency comb we measure a long term frequency instability of < 35 kHz for timescales between 10(-3) s and 10(3) s. As an application we perform spectroscopy of Sr Rydberg states from n = 37 - 81, demonstrating mode-hop-free scans of 24 GHz. In a cold atomic sample we measure Doppler-limited linewidths of 350 kHz.

Highlights

  • Tunable continuous-wave (CW) lasers are the workhorse for quantum technologies based on ultracold atoms and ions

  • In this paper we describe a solid-state, narrow-linewidth UV laser system tunable from 316.3 nm – 317.7 nm and 318.0 nm – 319.3 nm, which enables the two-step excitation of Sr Rydberg states with principal quantum number in the range n = 35 → > 300 from two different intermediate states that are separated by 5.6 THz

  • We considered both periodically-poled stoichiometric lithium tantalate (PPSLT) and periodically-poled lithium niobate (PPLN) crystals

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Summary

Introduction

Tunable continuous-wave (CW) lasers are the workhorse for quantum technologies based on ultracold atoms and ions. Most of these experiments have relied on a two-step excitation scheme via a shortlived, low-lying intermediate state While this has the advantage that both lasers may be in the visible or near-IR spectral regions, the short lifetime of the intermediate state introduces additional decoherence. An alternative approach to reducing the decoherence of the two-photon excitation scheme is provided by two-electron atoms such as Sr. Here, intercombination transitions give access to long-lived intermediate states. Intercombination transitions give access to long-lived intermediate states These provide a coherent two-photon excitation route to the triplet Rydberg states, including the 5sns 3S1 series which have near-isotropic wavefunctions and interaction strengths [24].

Laser construction and characterization
W 10 W f1a f1b D1 f2a f2b
Second harmonic generation to the UV
Laser frequency stabilization
Laser frequency characterization
Atomic spectroscopy
Conclusion
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