Abstract

We look into the quantum phase diagram of a spin- antiferromagnet on the square lattice with degenerate Shastry–Sutherland ground states, for which only a schematic phase diagram is known so far. Many exotic phases were proposed in the schematic phase diagram by the use of exact diagonalization on very small system sizes. In our present work, an important extension of this antiferromagnet is introduced and investigated in the thermodynamic limit using triplon mean-field theory. Remarkably, this antiferromagnet shows a stable plaquette spin-gapped phase like the original Shastry–Sutherland antiferromagnet, although both of these antiferromagnets differ in the Hamiltonian construction and ground state degeneracy. We propose a sublattice columnar dimer phase which is stabilized by the second and third neighbor antiferromagnetic Heisenberg exchange interactions. There are also some commensurate and incommensurate magnetically ordered phases, and other spin-gapped phases which find their places in the quantum phase diagram. Mean-field results suggest that there is always a level-crossing phase transition between two spin-gapped phases, whereas in other situations, either a level-crossing or a continuous phase transition happens.

Highlights

  • The emergence of exotic physical properties in strongly correlated systems is of great current interest [1,2,3,4,5]

  • J2 correspond to a spin singlet state and to three spin triplet states, respectively

  • The minimization of the ground state energy with respect to unknown mean-field parameters λ and s2 leads to selfconsistent equations which are solved as previously

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Summary

INTRODUCTION

The emergence of exotic physical properties in strongly correlated systems is of great current interest [1,2,3,4,5]. Motivated by the models with exact dimer ground states and the hidden challenges in the recently proposed deconfined quantum criticality, Gelle et al constructed a model which has an exact fourfold degenerate SS ground state (in contrast to the original SS model where there is no degeneracy) [41] This model consists of J1-J2 Heisenberg antiferromagnetic interactions and a multiple-spin exchange interaction K. Many other interesting magnetic and nonmagnetic phases emerge when energetically favorable conditions are met by tuning the interaction parameters The authors studied this model numerically using finite-size exact diagonalization, and presented a schematic quantum phase diagram. The exactly solvable limit of the model (1) is achieved when all J’s are set to zero Gelle et al [41]

TRIPLON MEAN-FIELD THEORY
Dimer triplon mean-field theory
Plaquette triplon mean-field theory
RESULTS
Quantum phase diagram in the J1-J2-K space
Quantum phase diagram in the J2-J3-K space

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