Abstract
Optical detection of zero-field magnetic resonance in the photoexcited triplet states of organic molecules requires a microwave-induced change in population among the triplet-state spin sublevels. The description of the dynamics of such triplet-state population changes in the presence of a microwave field is presented. This description provides a framework for obtaining intersystem crossing rate constants, and the results are discussed for fluorescence-, triplet absorption-, and singlet absorption-detected zero-field magnetic resonance spectroscopy.
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