Abstract
Summary Responses of commercial pH-sensitive and other cation-sensitive glass membranes have measured under application of voltage pulse steps and a.c. currents. Responses have been found to be independent of solution environment pH, alkali metal and magnitude of exciting signal over a wide range. Variations of response with temperature have been noted. The membranes acting as linear systems, respond in agreement with the theoretical predictions and verify the essential correctness of fixed site membrane theory applied to membrane transients. A range of behavior from ideal film-free pH glasses to highly hydrated film coated glass electrodes have been observed to test the extreme cases of the theory. Time constants and double-layer capacitances have been tabulated.
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