Abstract

Abstract. The important task to observe the global coverage of middle atmospheric trace gases like water vapor or ozone usually is accomplished by satellites. Climate and atmospheric studies rely upon the knowledge of trace gas distributions throughout the stratosphere and mesosphere. Many of these gases are currently measured from satellites, but it is not clear whether this capability will be maintained in the future. This could lead to a significant knowledge gap of the state of the atmosphere. We explore the possibilities of mapping middle atmospheric water vapor in the Northern Hemisphere by using Lagrangian trajectory calculations and water vapor profile data from a small network of five ground-based microwave radiometers. Four of them are operated within the frame of NDACC (Network for the Detection of Atmospheric Composition Change). Keeping in mind that the instruments are based on different hardware and calibration setups, a height-dependent bias of the retrieved water vapor profiles has to be expected among the microwave radiometers. In order to correct and harmonize the different data sets, the Microwave Limb Sounder (MLS) on the Aura satellite is used to serve as a kind of traveling standard. A domain-averaging TM (trajectory mapping) method is applied which simplifies the subsequent validation of the quality of the trajectory-mapped water vapor distribution towards direct satellite observations. Trajectories are calculated forwards and backwards in time for up to 10 days using 6 hourly meteorological wind analysis fields. Overall, a total of four case studies of trajectory mapping in different meteorological regimes are discussed. One of the case studies takes place during a major sudden stratospheric warming (SSW) accompanied by the polar vortex breakdown; a second takes place after the reformation of stable circulation system. TM cases close to the fall equinox and June solstice event from the year 2012 complete the study, showing the high potential of a network of ground-based remote sensing instruments to synthesize hemispheric maps of water vapor.

Highlights

  • Trace gases with a long chemical lifetime can serve as indicators for middle atmospheric dynamics

  • In this study we demonstrate that the trajectory mapping (TM) technique applied to ground-based water vapor profile measurements of a small instrument network operated within the frame of NDACC (Network for the Detection of Atmospheric Composition Change) has the ability to provide adequate information about the horizontal distribution of water vapor, even during fast changing dynamic conditions in the atmosphere (e.g., deformation of the stratospheric polar vortex during a stratospheric warming (SSW) event)

  • We conclude that the applied trajectory mapping technique (Sect. 2.4) is able to produce synoptic water vapor maps of high quality throughout stratospheric and mesospheric altiwww.atmos-chem-phys.net/15/9711/2015/

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Summary

Introduction

Trace gases with a long chemical lifetime can serve as indicators for middle atmospheric dynamics. In our study the focus is directed to middle atmospheric water vapor and its distribution in the Northern Hemisphere (NH). Chemical reactions like methane oxidation are the major source of middle atmospheric water vapor. These reactions happen in general below an altitude of 50 km (Brasseur and Solomon, 2006). In higher atmospheric regions the mean lifetime of water vapor due to vertical transport and photochemical mechanisms is similar and on the order of several weeks. As there is no other major chemical source of H2O in the mesosphere, it serves as an ideal tracer to study atmospheric dynam-

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