Abstract
We explore the formation of Ar hollow states with two or three inner-shell holes by free-electron-laser radiation. We find that even-charged Ar ion states can be more populated than odd-charged Ar ion states. This depends on the pulse intensity and the number of energetically accessible inner-shell holes. Fully accounting for fine structure, we demonstrate that one-electron spectra bear the imprints of Ar hollow states with two inner-shell holes. Moreover, we show how the Auger spectra of these hollow states can be extracted from two-electron coincidence spectra.
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