Abstract

Water vapor fluxes play a key role in the energy budget of the atmosphere, and better flux measurements are needed to improve our understanding of the formation of clouds and storms. Large-scale measurements of these fluxes are possible by employing the eddy correlation (EC) method from an aircraft. A hygrometer used for such measurements needs to deliver a temporal resolution of at least 10 Hz while reliably operating in the harsh conditions on the exterior of an aircraft. Here, we present a design concept for a calibration-free, first-principles, open-path dTDLAS hygrometer with a planar, circular and rotationally symmetric multipass cell with new, angled coupling optics. From our measurements, the uncertainty of the instrument is estimated to be below 4.5% (coverage factor k = 1). A static intercomparison between a dTDLAS prototype of the new optics setup and a traceable dew point mirror hygrometer was conducted and showed a systematic relative deviation of 2.6% with a maximal relative error of 2.2%. Combined with a precision of around 1 ppm H2O at tropospheric conditions, the newly designed setup fulfills the static precision and accuracy requirements of the proposed airborne EC hygrometer.

Highlights

  • Water vapor is the most important greenhouse gas, and plays a key role in the energy budget of the atmosphere [1]

  • The eddy correlation (EC) method can be used to measure these fluxes by correlating the vertical component of the wind vector with fast and accurate H2 O concentration values [3]

  • This method is commonly used in stationary setups, such as meteorological EC flux towers, to determine the water vapor flux from the ground into the atmosphere at one specific location [4,5]

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Summary

Introduction

Water vapor is the most important greenhouse gas, and plays a key role in the energy budget of the atmosphere [1]. The eddy correlation (EC) method can be used to measure these fluxes by correlating the vertical component of the wind vector with fast and accurate H2 O concentration values [3] This method is commonly used in stationary setups, such as meteorological EC flux towers, to determine the water vapor flux from the ground into the atmosphere at one specific location [4,5]. The use of a closed- or open-path optical cell is one of the key characteristics of an airborne hygrometer. Notable instruments that utilize an extractive sampling and a closed-path cell on are [6,7,9,10,11,12,13,14,15,16,17].

Methods
Methodology
Optics Design
Uncertainty
Static Validation with a Dew Point Mirror and Spectroscopic Performance
All observed deviations are mum relative deviation between is
Correlation
Conclusions and AirborneApplication
OAirborne
Findings
Explosion view ofofthe airbornedTDLAS
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