Abstract

Graphene/CNTs-reinforced alumina ceramic composites were prepared by spark plasma sintering (SPS) method at 1500 °C. The distribution behaviors of graphene/CNTs reinforcements in alumina matrix composite were studied and mechanical properties of the composite were tested. The structural integrity of the graphene after sintering was analyzed by Raman spectroscopy. The composites show inter and trans-granular fracture behaviors. Many toughening mechanisms such as graphene and CNTs necking, crack bridging, crack deflection and crack branching were observed. The experiment-based calculation of heat capacity of the composite was presented in details. The thermal diffusivity and thermal conductivity of the nanocomposites were discussed. The thermal conductivity increased with the increase of grain size. The pure alumina had the highest thermal conductivity, which was 23.9 Wm−1 K−1.

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