Time-resolved X-ray Diffraction Studies of Coherent Lattice Dynamics Using Synchrotron Radiation

Abstract

Significant progress in recent development of synchrotron radiation (SR) sources has offered the opportunity for time-resolved X-ray diffraction studies of fast lattice dynamics in the atomic scale. The coherent atomic motion, as seen in coherent optical and acoustic phonons which are induced by femtosecond pulsed laser irradiation of semiconductor surface has directly been observed with the time-resolved X-ray diffraction technique. In this article, the time-resolved diffraction methods using an SR beam are summarized, and the demonstrations for acoustic pulse echo, coherent acoustic phonon, and optical phonon are reviewed as examples of the investigation on coherent lattice dynamics. The future prospective on the investigation of lattice dynamics using time-resolved X-ray diffraction experiments is also discussed.