Abstract
Is an atom more likely to scatter a photon with an exponentially rising or decaying temporal profile? We try to answer this question experimentally and investigate the scattering of heralded photons from a single atom in free-space [1]. We use a single Rubidium atom trapped in optical tweezers and prepared in the groundstate of a cyclic dipole transition as a textbook-like two-level system. A time-ordered photon pair source, in conjunction with an asymmetric cavity, generates heralded single photons with an exponentially decaying or rising temporal profile [2, 3]. The heralded photons are resonant with the atomic transition and have a bandwidth comparable to the atomic linewidth. The photons are strongly focused onto the atom by a large numerical aperture lens. We study the scattering dynamics by measuring the atomic emission and the reduction in the number of transmitted photons. We perform the scattering experiment for photons with exponentially decaying and rising temporal envelopes and find that the atomic dynamics depend on the temporal profile of the photon. The atomic absorption is shorter but has a higher maximum for the rising photon than for the the decaying one. Interestingly, the overall probability that the photon is scattered by the atom is similar for decaying and rising photons.
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