Abstract

With minor modifications to commercial instrumentation, time-resolved FTIR emission spectroscopy is demonstrated for the determination of photofragment internal state distributions. Vinyl chloride and dichloroethylene photolysis at 193 nm serve as test cases and exhibit high signal-to-noise. The vibrational distributions in the first four levels of the HCl photo-product of vinyl chloride and 1,2-trans-dichloroethylene are in good agreement with previous determinations.

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