Abstract
A time-dependent quantum dynamics theory has been presented to interpret product partial cross-sections of the photofragmentation of triatomic molecule by treating correctly the coupling of angular momenta and taking fully into account the vector properties of the transition dipole moment and electric field of the exciting radiation. A model system of [Formula: see text] has been used to study the nuclear motion of N 2 photofragments through the asymptotic dissociation channels which relies upon the transition dipole vector either lies parallel on the molecular plane (1A′→1A′) or perpendicular to the molecular plane (1A′→1A′′).
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