Abstract

Intermediate states of the two-photon ionization of the three aromatic molecules in cyclohexane were investigated using a time-delayed two-color technique. The S 1 state is a major intermediate for the two-photon ionization of anthracene and benzo [a] pyrene, while both the S 1 and S 2 states are intermediates for pyrene. Ionization through the short-lived S 2 state was enhanced through autoionization resonance.

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